The Journal of chemical physics
Unified theory of internal conversion and fluorescence under macroscopic quantum electrodynamics framework.
Chih-En Shen, Hung-Sheng Tsai, Liang-Yan Hsu
Published: 202510.1063/5.0299368
Abstract
We develop a unified first-principles formulation of fluorescence and internal conversion (IC) within the framework of macroscopic quantum electrodynamics (QED). For molecules with negligible spin-orbit coupling, the approach accounts for both radiat…
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