Rational construction of donor-acceptor covalent heptazine polymers for efficient photocatalytic N2 reduction to NH3.

Three novel donor-acceptor covalent heptazine polymers were rationally constructed by regulating the donor and the electronic structure of the acceptor. The results show that the photocatalytic N2 reduction to NH3 of Cy-Tq is up to 562 µmol g-1 h-1 t…

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