Journal of the American Chemical Society
Tunable Multisite Proton-Coupled Electron Transfer Mediators: Distinct Pathways for Substrate Reduction Versus Competing Hydrogen Evolution.
John M Ovian, Joseph Derosa, Mengdi Li, Jonas C Peters
Published: 202610.1021/jacs.5c18522
Abstract
Proton-coupled electron transfer (PCET) reagents have emerged as powerful tools for transferring net H atoms to organic substrates from relatively weak X-H bonds. One advantage of employing PCET reagents is the tunability of the X-H bond strength by…
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