Journal of the American Chemical Society
Insights into the Active Sites for Catalytic Steam Reforming of Methane from Oscillations in the Reaction.
Yu Zhang, Qian Wang, Peter Glarborg, Martin P Andersson, Jakob B Wagner, Keld Johansen, Thomas K Torp, Jean-Claude Grivel, Anker D Jensen, Chaofeng Hou, Wei Ge, Jakob M Christensen
Published: 202510.1021/jacs.5c11696
Abstract
A new oscillating catalytic reaction is discovered: steam reforming of CH4 in the presence of SO2 over Rh nanoparticles. The reducing products from the reforming reaction convert SO2 to adsorbed sulfur, which causes deactivation. When activity, and t…
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